William Dieterle
Valentin (archive footage)
Gösta Ekman
Himself / Faust (archive footage)
Yvette Guilbert
Marthe Schwerdtlein (archive footage)
Camilla Horn
Herself / Gretchen (archive footage)
Emil Jannings
Himself / Mephisto (archive footage)
F. W. Murnau
Himself (archive footage)
Frida Richard
Gretchen's mother (archive footage)
Werner Fuetterer
Archangel (archive footage) (uncredited)
Ana Cristina Iriarte
Voice (Narrator)